3.31 to 3.73 worth it?

Hello all! Will it be worth the work changing from 3.31 to 3.73 ratio? I have the 741 center and the 3.73 is the "biggest" gear I can find for that center. I want to be quicker of the line. Also played with the thought of changing to a higher stall converter.

My current combo:
1965-273
727
340 Cam
Edelbrock D4B intake / Edelbrock 600 Performer Carb
Headers
2.5" Dual Exhaust
8 3/4 - 3.31 - SureGrip