Would this brake conversion work?

Just for information: I have to change everything on the brakes anyway. The car stood 20 years

Unless you change to the larger brake shoes, 1) I am not sure the larger cylinders will FIT and 2) you will see very little difference. I bought my 64 Valiant in January that had sat since 1982. That was the first thing I did after I got the engine running was rebuild the brakes. Mine has the 9" drums all around and it stops very well.