Charging issues on a ‘64 Valiant...

If you have an alternator with both horizontal and vertical brushes in plastic holders, then you can replace the parts and convert the wiring so it works with that type of regulator. Or you still have the option of grounding one and using a positive controlling regulator.
I posted a crib sheet for the replacement brushes and holders here:
Alternator repair, a little show and tell.

That is the same exact one is mine. I used the picture off Amazon because it’s raining. Both brushes are there, but if you see the one on the left has the full spade connector and a black washer and the one on the right has the tip of spade clipped off with no washer. I believe I may be able to convert it back thanks to the help on here.