Improving acceleration using 2bbl Carburetor?

It's a 270 /6. How do I adjust valves and "baseline" the car back to tune, and what tools would I need?

Look at post № 11 in this thread (on the first page). Wherever you see boldface, blue type, that's a clickable link. Click it to go to the information it represents. As you are new to all this, as soon as you can, get the three books listed in this thread.


I want to get it to running its best and then figure out what to do from there

Wise. See this thread about that.

Note there is nothing such as a 270 Slant-6. "270" is the model series of your Dart. The 170 was the basic/low-trim series. The 270 was the high-trim series. The GT was the premium series. It's a little confusing because the standard-equipment engine was a 170 cubic inch Slant-6, but any Dart model could be had with any of the available engines. Your engine is either a 170 or a 225 Slant-6. Look at the driver's side of the engine block, below/behind the manifolds. What casting numbers do you see?