Cooling Issue - 1964 Dart GT - 273 with automatic and A/C

A properly designed and build shroud can be very effective. If the OP isn't worried about originality, I'd make one that directs almost all the air through the radiator. Some sheet metal and rubber sheets cut to fit and riveted/bolted in the right places could do wonders.
Agreed, but the original shroud looks really sketchy.